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Polarization spectroscopy of positive and negative trions in an InAs quantum dot

Identifieur interne : 000351 ( Russie/Analysis ); précédent : 000350; suivant : 000352

Polarization spectroscopy of positive and negative trions in an InAs quantum dot

Auteurs : RBID : Pascal:05-0153583

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English descriptors

Abstract

Using polarization-sensitive photoluminescence and photoluminescence excitation spectroscopy, we study single InAs/GaAs self-assembled quantum dots. The dots were embedded in an n-type, Schottky diode structure allowing for control of the charge state. We present here the exciton, singly charged exciton (positive and negative trions), and the twice negatively charged exciton. For non-resonant excitation below the wetting layer, we observed a large degree of polarization memory from the radiative recombination of both the positive and negative trions. In excitation spectra, through the p-shell, we have found several sharp resonances in the emission from the s-shell recombination of the dot in all charged states. Some of these excitation resonances exhibit strong coulomb shifts upon addition of charges into the quantum dot. One particular resonance of the negatively charged trion was found to exhibit a fine structure doublet under circular polarization. This observation is explained in terms of resonant absorption into the triplet states of the negative trion.

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Pascal:05-0153583

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<name sortKey="Gershoni, David" uniqKey="Gershoni D">David Gershoni</name>
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<name sortKey="Korenev, Vladimir L" uniqKey="Korenev V">Vladimir L. Korenev</name>
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<term>Gallium arsenides</term>
<term>Indium arsenides</term>
<term>Photoluminescence</term>
<term>Quantum dots</term>
<term>Radiative recombination</term>
<term>Schottky barriers</term>
<term>Self-assembled layers</term>
<term>Semiconductor materials</term>
<term>Trion</term>
<term>Triplet state</term>
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<term>Polarisation circulaire</term>
<term>Trion</term>
<term>Photoluminescence</term>
<term>Barrière Schottky</term>
<term>Exciton</term>
<term>Recombinaison radiative</term>
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<div type="abstract" xml:lang="en">Using polarization-sensitive photoluminescence and photoluminescence excitation spectroscopy, we study single InAs/GaAs self-assembled quantum dots. The dots were embedded in an n-type, Schottky diode structure allowing for control of the charge state. We present here the exciton, singly charged exciton (positive and negative trions), and the twice negatively charged exciton. For non-resonant excitation below the wetting layer, we observed a large degree of polarization memory from the radiative recombination of both the positive and negative trions. In excitation spectra, through the p-shell, we have found several sharp resonances in the emission from the s-shell recombination of the dot in all charged states. Some of these excitation resonances exhibit strong coulomb shifts upon addition of charges into the quantum dot. One particular resonance of the negatively charged trion was found to exhibit a fine structure doublet under circular polarization. This observation is explained in terms of resonant absorption into the triplet states of the negative trion.</div>
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<s0>Using polarization-sensitive photoluminescence and photoluminescence excitation spectroscopy, we study single InAs/GaAs self-assembled quantum dots. The dots were embedded in an n-type, Schottky diode structure allowing for control of the charge state. We present here the exciton, singly charged exciton (positive and negative trions), and the twice negatively charged exciton. For non-resonant excitation below the wetting layer, we observed a large degree of polarization memory from the radiative recombination of both the positive and negative trions. In excitation spectra, through the p-shell, we have found several sharp resonances in the emission from the s-shell recombination of the dot in all charged states. Some of these excitation resonances exhibit strong coulomb shifts upon addition of charges into the quantum dot. One particular resonance of the negatively charged trion was found to exhibit a fine structure doublet under circular polarization. This observation is explained in terms of resonant absorption into the triplet states of the negative trion.</s0>
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